Upconversion Detection for Improved Nonlinear Mid-infrared Spectroscopy in Flames
This thesis deals with the addition of upconversion detection to non-linear mid-infrared laser spectroscopy techniques. The techniques investigated here are degenerate four wave mixing (DFWM) and infrared polarization spectroscopy (IRPS). These techniques are useful for detecting many of the key species in combustion, such as CH4, C2H6, HCl, and HCN. These species can be probed using ro-vibrationa
