Rotational Coherent Anti-Stokes Raman Spectroscopy: Experimental and Theoretical Developments in Gas-phase Thermometry
Dual-broadband pure rotational coherent anti-Stokes Raman spectroscopy was investigated in terms of thermometry and species concentration measurement for studies of combustion. The modelling of rotational CARS spectra under conditions of high pressure at room temperature was investigated. Resonant terms of the Stokes (CSRS) type were found to have a significant effect on the intensity of the anti